论文标题

使用TiO2的模板原子层沉积在钻石膜上的高Q纳米光谐振器

High-Q Nanophotonic Resonators on Diamond Membranes using Templated Atomic Layer Deposition of TiO2

论文作者

Butcher, Amy, Guo, Xinghan, Shreiner, Robert, Delegan, Nazar, Hao, Kai, Duda III, Peter J., Awschalom, David D., Heremans, F. Joseph, High, Alexander A.

论文摘要

将固态量子发射器与纳米光谐振器集成,对于有效的自旋式接口和光学网络应用至关重要。尽管事实证明,钻石颜色中心是新兴量子技术的出色候选者,但它们与光谐振器的集成仍然具有挑战性。基于将谐振器蚀刻到钻石中的传统方法通常会对颜色中心的性能产生负面影响,并提供较低的设备产量。在这里,我们基于钻石膜上TIO2的模板原子层沉积开发了一个集成的光子平台。我们的制造方法产生了高性能的纳米光子设备,同时避免将波长尺度刻在钻石中。此外,该技术会产生高度可重现的光学共振,并且可以在单个钻石样品上迭代,这是一个独特的处理优势。我们的方法适用于各种波长和底物,可以在钻石或碳化硅,稀土离子或其他材料系统中在腔光光子或相干缺陷之间进行高共接口。

Integrating solid-state quantum emitters with nanophotonic resonators is essential for efficient spin-photon interfacing and optical networking applications. While diamond color centers have proven to be excellent candidates for emerging quantum technologies, their integration with optical resonators remains challenging. Conventional approaches based on etching resonators into diamond often negatively impact color center performance and offer low device yield. Here, we developed an integrated photonics platform based on templated atomic layer deposition of TiO2 on diamond membranes. Our fabrication method yields high-performance nanophotonic devices while avoiding etching wavelength-scale features into diamond. Moreover, this technique generates highly reproducible optical resonances and can be iterated on individual diamond samples, a unique processing advantage. Our approach is suitable for a broad range of both wavelengths and substrates and can enable high-cooperativity interfacing between cavity photons and coherent defects in diamond or silicon carbide, rare earth ions, or other material systems.

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