论文标题
在量子审查下有限温度下的2D铁磁性
2D ferromagnetism at finite temperatures under quantum scrutiny
论文作者
论文摘要
近年来,二维(2D)磁性材料的巨大升高,其中一些磁性材料通过实验验证。但是,迄今为止的大多数理论预测都取决于在零温度和无波动下的AB-Initio方法,而当然可以期望在有限温度下发生有害的量子波动。在这里,我们介绍了与蜂窝/六角形晶格量子模型的解决方案,具有各向异性交换相互作用,最多是第三位最近的邻居,并且在任意方向上的应用领域中,该问题回答了远距离磁化的问题,是否确实可以在材料的超层次限制中生存在材料的超级限制中,以达到哪个温度,以及磁性的磁性(量强度)的材料(量强度)。我们发现,对于具有整体易于轴各向异性的材料,在有限温度下,远距离磁性秩序持续存在。我们验证了单层CRI3,CRBR3和MNSE2的示例的计算。此外,我们提供了一种易于使用的工具来计算新2D计算材料的居里温度。
Recent years have seen a tremendous rise of two-dimensional (2D) magnetic materials, several of which verified experimentally. However, most of the theoretical predictions to date rely on ab-initio methods, at zero temperature and fluctuations-free, while one certainly expects detrimental quantum fluctuations at finite temperatures. Here we present the solution of the quantum Heisenberg model for honeycomb/hexagonal lattices with anisotropic exchange interaction up to third nearest neighbors and in an applied field in arbitrary direction, that answers the question whether long-range magnetization can indeed survive in the ultrathin limit of materials, up to which temperature, and what the characteristic excitation (magnon) frequencies are, all essential to envisaged applications of magnetic 2D materials. We find that long-range magnetic order persists at finite temperature for materials with overall easy-axis anisotropy. We validate the calculations on the examples of monolayer CrI3, CrBr3 and MnSe2. Moreover, we provide an easy-to-use tool to calculate Curie temperatures of new 2D computational materials.