论文标题

磁性大量光伏效应:强场和弱场

Magnetic Bulk Photovoltaic Effect: Strong and Weak Field

论文作者

Dai, Zhenbang, Rappe, Andrew M.

论文摘要

已经提出了移位电流和弹道电流来解释大量光伏效应(BPVE),并进行了实验旨在分离两种机制。这些实验是基于这样的假设:在磁场下,弹道电流可以具有霍尔效应,而移位电流不能,这是来自某些能量尺度参数,并且从未得到证明。最近的工作[物理学。 Rev. B 103,195203(2021)使用量子运输形式主义得出的结论是,Shift电流确实具有霍尔电流,似乎与先前的假设相矛盾,并使情况更加混乱。此外,在强磁场下BPVE的行为仍未开发。在这封信中,使用最小的2D紧密结合模型,我们通过以非扰动方式处理弱磁场下的BPVE进行系统的数值研究。我们的模型清楚地显示了沿横向磁性诱导的弹道电流的外观,这与先前的预测一致,有趣的是,也观察到了移位电流的相当大的纵向响应,这种现象均未被任何现有理论所捕获的现象,在该现象中,磁场是在磁场上被触流的。更令人惊讶的是,在强场状态中发现了截然不同的移位电流,并且从弱场到强场的演变类似于相变。我们希望我们的工作能够解决有关磁场下BPVE行为的争论,并且有望启发更多关于非线性光学和量子几何形状之间关系的研究的强场行为。

Shift current and ballistic current have been proposed to explain the bulk photovoltaic effect (BPVE), and there have been experiments designed to separate the two mechanisms. These experiments are based on the assumption that under magnetic field, ballistic current can have a Hall effect while the shift current cannot, which is from some energy-scale arguments and has never been proven. A recent work [Phys. Rev. B 103, 195203 (2021)] using quantum transport formalism achieves a conclusion that shift current indeed has a Hall current, seemingly contradicting the previous assumption and making the situation more confusing. Moreover, the behavior of BPVE under strong magnetic field is still unexplored. In this Letter, using a minimal 2D tight-binding model, we carry out a systematic numerical study of the BPVE under weak and strong magnetic field by treating the field in a non-perturbative way. Our model clearly shows the appearance of the magnetically-induced ballistic current along the transverse direction, which agrees with the previous predictions, and interestingly a sizable longitudinal response of the shift current is also observed, a phenomenon that is not captured by any existing theories where the magnetic field is treated perturbatively. More surprisingly, drastically different shift current is found in the strong-field regime, and the evolution from weak to strong field resembles a phase transition. We hope that our work could resolve the debate over the behavior of BPVE under magnetic field, and the strong-field behavior of shift current is expected to inspire more studies on the relation between nonlinear optics and quantum geometry.

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